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Theoretical Analysis of the Carrier Concentration Effect of the EAU
——————————————————————-

Based on the results of the measurements mentioned above, the carrier concentration effect of the EAU on EQE has been theoretically analyzed ([Figure 7](#F7){ref-type=”fig”}). Under the condition that the ambipolar EEs of the donor (D) and the acceptor (A) were the same, the EQE was shown to have a minimum value of 50% at an optimal *N* of \~2.4 × 10^17^ cm^−3^. This result is attributed to the fact that the optimization of the average energy level of the bandgap is very important for achieving the maximum EQE. Since the doping concentration of the EAU is used to shift the average energy level of the bandgap, the positive effect on the EQE is proportional to the carrier concentration of the EAU. The results of the theoretical analysis of the carrier concentration effect of the EAU are in good agreement with the experimental observations.

![Comparison between the theoretical prediction and the experimental EQE under the condition that the ambipolar energy level of D and A were the same.](fchem-07-00818-g0007){#F7}

Conclusion {#s4}
==========

In summary, we have shown that a new type of ambipolar A-D heterojunction with the structure of PAQZ-NPB-ZnO-EAU has a distinct positive effect on the EQE. The positive effect of the new A-